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Answer to Question #1794 Submitted to "Ask the Experts"Category: Radiation Effects — Effects on Materials The following question was answered by an expert in the appropriate field: Q
I'm asking for research information to help me to assess the potential consequences of a chemical fire involving the most utilized radioactive sealed sources in chemical industry. Most of these sources contain 63Ni, 60Co, 137Cs, 192Ir, and 241Am with an activity of ~3.7 Gbq. The reason is that with new laws in Belgium, every company has to make an emergency plan (a worst-case scenario) for every installation that utilizes radioactive sources. Until now I haven't found any publication or study concerning (1) how these containers and source capsules respond to a serious chemical fire, say 1,000o C for more than one hour, (2) the chance of release of radioactive material by the sealed sources, (3) the resulting dose at different distances from the sources when radioactive material is released, (4) if there is release of radioactive material, what distances should be observed by employees, workforce, firefighters, and emergency personnel to be sure exposure limits could not be exceeded, (5) how these radioactive materials release in the atmosphere due to the fire and to what distance to the smoke plume evacuation could be expected, and (6) I've been told that the source capsule is subject to norms but not the lead container, which contains the capsule. Is this correct and why? If any literature exists, could you give me the references?
A
The following information was compiled and edited from information provided by William Ward and Douglas Broaddus of the United States Nuclear Regulatory Commission (NRC). ISO 2919 is the international standard for sealed sources. The manufacturer of a device makes a determination as to the maximum heat a device is likely to see during accident and normal conditions, and selects sources to meet that condition. The highest classification, temperature-wise, is a 6, and that is 800o C for 1 hour. In other words, if a manufacturer chose a source rated at 6 for temperature, it should last for 1 hour at 800o C without its boundary failing. Anything beyond that requires special testing and classification. There won't be many sources designed for a more extreme temperature condition. There is no testing for chemical conditions such as an acid/caustic environment. Generally, the system is designed to avoid placing a source in such conditions. But such a condition may arise in an accident scenario. Generally, it is assumed that any lead will melt away in a fire (structural containment of lead is assumed to have failed), so it is not included in shielding calculations in fire situations. Other testing of sources, required by ISO 2919, can give an idea as to the method and likelihood of failure of the source containment (over-pressurization, impact, etc.) for various postulated situations. It is up to the applicant to propose likely extreme situations and how they would be handled. For a 1,000o C chemical fire for 1 hour, an applicant would likely assume lead is gone and containment has failed and discuss a measured approach to fighting the fire and source recovery. This would likely be based on health physics principles since engineering designs have failed. However, in a fresh reactor fuel fire in Springfield, Massachusetts, they let it burn rather than put water on it. The fear was thermally shocking the metal, causing it to fail. The responders decided it would likely survive the fire, since it had up to the point when the decision was made. In general, the NRC does not specify requirements concerning accident analysis. We expect the applicant to propose scenarios and explain why they don't present a problem that would prevent the NRC from issuing the certificate of registration [see Title 10 of the United States Code of Federal Regulations Part 32.210(c) & (d)]. The only example of a health physics-based analysis similar to this situation that could be readily found is in the NRC regulatory guidance document NUREG-1556, Volume 8, Appendix O, Attachment 1. NUREG 1556, Volume 3 "Applications for Sealed Source and Device Evaluation and Registration," also provides a more general description of NRC's approach to evaluating SS&D registration applications. In particular, Appendix F "Standard Reference Materials," lists various reference documents typically used during the evaluation process. The NUREG 1556 series is available on the NRC Web site. Volume 3 and Volume 8 are also available on the NRC Web site. Keith Dinger, CHP
Answer posted on 15 May 2002. The information and material posted on this Web site is intended as general reference information only. Specific facts and circumstances may alter the concepts and applications of materials and information described herein. The information provided is not a substitute for professional advice and should not be relied upon in the absence of such professional advice specific to whatever facts and circumstances are presented in any given situation. Answers are correct at the time they are posted on the Web site. Be advised that over time, some requirements could change, new data could be made available, or Internet links could change. For answers that have been posted for several months or longer, please check the current status of the posted information prior to using the responses for specific applications.
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